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  • NEANIAS Atmospheric Research Community
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Gabriel Pasquet; Rokiya Houssein Hassan; Olivier Sissmann; Jacques Varet; +1 Authors

    Dihydrogen (H2) is generated by fluid–rock interactions along mid-ocean ridges (MORs) and was not, until recently, considered as a resource. However, in the context of worldwide efforts to decarbonize the energy mix, clean hydrogen is now highly sought after, and the production of natural H2 is considered to be a powerful alternative to electrolysis. The Afar Rift System has many geological features in common with MORs and offers potential in terms of natural H2 resources. Here, we present data acquired during initial exploration in this region. H2 contents in soil and within fumaroles were measured along a 200 km section across the Asal–Ghoubbet rift and the various intervening grabens, extending from Obock to Lake Abhe. These newly acquired data have been synthesized with existing data, including those from the geothermal prospect area of the Asal–Ghoubbet rift zone. Our results demonstrate that basalt alteration with oxidation of iron-rich facies and simultaneous reduction in water is the likely the source of the hydrogen, although H2S reduction cannot be ruled out. However, H2 volumes at the surface within fumaroles were found to be low, reaching only a few percent. These values are considerably lower than those found in MORs. This discrepancy may be attributed to bias introduced by surface sampling; for example, microorganisms may be preferentially consuming H2 near the surface in this environment. However, the low H2 generation rates found in the study area could also be due to a lack of reactants, such as fayalite (i.e., owing to the presence of low-olivine basalts with predominantly magnesian olivines), or to the limited volume and slow circulation of water. In future, access to additional subsurface data acquired through the ongoing geothermal drilling campaign will bring new insight to help answer these questions.

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    Geosciences
    Other literature type . Article . 2021 . Peer-reviewed
    License: CC BY
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    Geosciences
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    Geosciences
    Article . 2022
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Geosciencesarrow_drop_down
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      Other literature type . Article . 2021 . Peer-reviewed
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      Article . 2022
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Aguilar, M.; Ali Cavasonza, Leila; Behlmann, M.; Laudi, E.; +197 Authors

    Physical review letters 127(27), 271102 (2021). doi:10.1103/PhysRevLett.127.271102 Published by APS, College Park, Md.

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    CERN Document Server
    Other literature type . 2021
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    Physical Review Letters
    Article . 2021
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    Physical Review Letters
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    Article . 2021
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    Physical Review Letters
    Article . 2021 . Peer-reviewed
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    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
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    Article . 2021
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    Article . 2021
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Archivio Istituziona...arrow_drop_down
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
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      CERN Document Server
      Other literature type . 2021
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      Article . 2021
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      Article . 2021 . Peer-reviewed
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      Article . 2021
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Laura Martel; Thibault Charpentier; Pedro Amador Cedran; Chris Selfslag; +4 Authors

    In this study we reported the synthesis of three polycrystalline uranium borides UB1.78±0.02, UB3.61±0.041, and UB11.19±0.13 and their analyses using chemical analysis, X-ray diffraction, SQUID magnetometry, solid-state NMR, and Fourier transformed infrared spectroscopy. We discuss the effects of stoichiometry deviations on the lattice parameters and magnetic properties. We also provide their static and MAS-NMR spectra showing the effects of the 5f-electrons on the 11B shifts. Finally, the FTIR measurements showed the presence of a local disorder.

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      Article . 2021 . Peer-reviewed
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    Authors: D.-D. Rousseau; D.-D. Rousseau;

    When addressing the nature and origin of loess deposits and the associated environment as deduced from terrestrial mollusc faunas, Vojen Ložek produced a synthetic review of the state of the art at that time (Ložek, 1965a). This synthesis was one among several papers that he published the same year in English about “The loess environment in Central Europe” (Ložek, 1965c) or “Problems of analysis of the Quaternary nonmarine molluscan fauna in Europe” (Ložek, 1965b). It was mainly based on his own experience of investigating terrestrial molluscs in Czechoslovakian Quaternary deposits.

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    Copernicus Publications
    Other literature type . 2021
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    Eiszeitalter und Gegenwart
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    Eiszeitalter und Gegenwart
    Article . 2021 . Peer-reviewed
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    https://doi.org/10.7916/d8-6cw...
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    Authors: N. Deabji; N. Deabji; K. W. Fomba; S. El Hajjaji; +4 Authors

    Field measurements were conducted to determine aerosol chemical composition at a newly established remote high-altitude site in North Africa at the Atlas Mohammed V (AMV) atmospheric observatory located in the Middle Atlas Mountains. The main objectives of the present work are to investigate the variations in the aerosol composition and better assess global and regional changes in atmospheric composition in North Africa. A total of 200 particulate matter (PM10) filter samples were collected at the site using a high-volume (HV) collector in a 12 h sampling interval from August to December 2017. The chemical composition of the samples was analyzed for trace metals, water-soluble ions, organic carbon (OC/EC), aliphatic hydrocarbons, and polycyclic aromatic hydrocarbon (PAH) contents. The results indicate that high-altitude aerosol composition is influenced by both regional and transregional transport of emissions. However, local sources play an important role, especially during low wind speed periods, as observed for November and December. During background conditions characterized by low wind speeds (avg. 3 m s−1) and mass concentrations in the range from 9.8 to 12 µg m−3, the chemical composition is found to be dominated by inorganic elements, mainly suspended dust (61 %) and ionic species (7 %), followed by organic matter (7 %), water content (12 %), and unidentified mass (11 %). Despite the proximity of the site to the Sahara, its influence on the atmospheric composition at this high-altitude site was mainly seasonal and accounted for only 22 % of the sampling duration. Biogenic organics contributed up to 7 % of the organic matter with high contributions from compounds such as heneicosane, hentriacontane, and nonacosane. The AMV site is dominated by four main air mass inflows, which often leads to different aerosol chemical compositions. Mineral dust influence was seasonal and ranged between 21 % and 74 % of the PM mass, with peaks observed during the summer, and was accompanied by high concentrations of SO42- of up to 3.0 µg m−3. During winter, PM10 concentrations are low (<30 µg m−3), the influence of the desert is weaker, and the marine air masses (64 %) are more dominant with a mixture of sea salt and polluted aerosol from the coastal regions (Rabat and Casablanca). During the daytime, mineral dust contribution to PM increased by about 42 % because of road dust resuspension. In contrast, during nighttime, an increase in the concentrations of alkanes, PAHs, alkane-2-ones, and anthropogenic metals such as Pb, Ni, and Cu was found due to variations in the boundary layer height. The results provide the first detailed seasonal and diurnal variation of the aerosol chemical composition, which is valuable for long-term assessment of climate and regional influence of air pollution in North Africa.

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    Atmospheric Chemistry and Physics (ACP)
    Article . 2021 . Peer-reviewed
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    Article . 2021
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      Atmospheric Chemistry and Physics (ACP)
      Article . 2021 . Peer-reviewed
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      Article . 2021
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    Authors: Benjamin Pohl; Vincent Favier; Jonathan Wille; Danielle G. Udy; +8 Authors

    AbstractHere, we define weather regimes in the East Antarctica—Southern Ocean sector based on daily anomalies of 700 hPa geopotential height derived from ERA5 reanalysis during 1979–2018. Most regimes and their preferred transitions depict synoptic‐scale disturbances propagating eastwards off the Antarctic coastline. While regime sequences are generally short, their interannual variability is strongly driven by the polarity of the Southern Annular Mode (SAM). Regime occurrences are then intersected with atmospheric rivers (ARs) detected over the same region and period. ARs are equiprobable throughout the year, but clearly concentrate during regimes associated with a strong atmospheric ridges/blockings on the eastern part of the domain, which act to channel meridional advection of heat and moisture from the lower latitudes towards Antarctica. Both regimes and ARs significantly shape climate variability in Antarctica. Regimes favorable to AR occurrences are associated with anomalously warm and humid conditions in coastal Antarctica and, to a lesser extent, the hinterland parts of the Antarctic plateau. These anomalies are strongly enhanced during AR events, with warmer anomalies and dramatically amplified snowfall amounts. Large‐scale conditions favoring AR development are finally explored. They show weak dependency to the SAM, but particularly strong atmospheric ridges/blockings over the Southern Ocean appear as the most favorable pattern, in which ARs can be embedded, and to which they contribute.

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    Journal of Geophysical Research Atmospheres
    Article . 2021 . Peer-reviewed
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    Article . 2021
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      Journal of Geophysical Research Atmospheres
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    Authors: Lemenkova, Polina;

    Zusammen mit der Entwicklung der Skripttechnologie in der Kartographie, wie den Generic Mapping Tools (GMT) und Bibliotheken der Programmiersprache R, wird die geologische und geophysikalische Kartierung energisch vorangetrieben, wobei die Integration der thematischen Daten, wie GEBCO/SRTM, EGM-2008 und offene geologische Raster- und Vektorschichten sind einer der primären Datensätze, die hochauflösende Rohquellen für die kartografische Visualisierung in geologisch komplexen Regionen wie Pakistan liefern. Diese Studie zielt darauf ab, Skriptmethoden der automatisierten Kartographie, Methoden der angewandten Geoinformatik für die geomorphometrische Analyse und technische Datenverarbeitung (Formatierung, Projektion, Darstellung) zu integrieren, um eine Synthese der geologischen, geophysikalischen und geomorphologischen Karten Pakistans als neue Informationen zur Unterstützung der Analyse bereitzustellen der georäumlichen Variationen von Geologie, Geomorphologie, Tektonik und Schwerkraftfeldern mit besonderem Schwerpunkt auf der geologisch bemerkenswerten Region Pakistan: Sulaiman Fold Belt und Muslim Bagh Ophiolith-Komplex. Diese Studie stellt neue 12 thematische Karten vor, die technisch mithilfe von Skriptansätzen und offenen Tools erstellt werden. Alle Karten decken die Region Pakistan ab und werden mit Open-Source-Tools erstellt: GMT, R und QGIS. Für die Kartierung Pakistans wird eine GMT- und R-basierte Skriptzuordnung angewendet, deren Algorithmusschritte schrittweise als Codeausschnitte dargestellt werden. Basierend auf der Kombination von Programmier- und Skripttechniken und mit zusätzlicher QGIS-basierter Kartierung wird ein systemkomplexer Ansatz zur Datenintegration und Formatumgestaltung, Datenkonvertierung und Neuformatierung für ein einzelnes Projekt zur Geologie Pakistans entworfen und entwickelt, das die Daten effektiv integriert thematische Geodatensätze mit mehreren Ursprüngen. Um die beste Visualisierung zu erreichen, wurden verschiedene Farbpaletten und kartografische Visualisierungsansätze verwendet. Die resultierenden Karten werden erklärt und diskutiert. Zusammenhänge zwischen räumlichen Phänomenen der Schwerkraft der Erde, geologischer Entwicklung und tektonischen Bewegungen wurden aufgezeigt und kommentiert. Neue 12 Karten präsentieren die regionale geologische Lage des Landes. Along with the development of the scripting technology in cartography, such as the Generic Mapping Tools (GMT) and libraries of R programming language, geologic and geophysical mapping is being vigorously promoted, where the integration of the thematic data, such as GEBCO/SRTM, EGM-2008 and open geological raster and vector layers is one of the primary datasets that provides the high- resolution raw sources for cartographic visualization in the geologically complex regions like Pakistan. This study aims to integrate scripting methods of automated cartography, methods of applied geoinformatics for geomorphometric analysis and technical data processing (formatting, projecting, plotting), to provide a synthesis of the geological, geophysical and geomorphological maps of Pakistan they as new information supporting analysis of the geospatial variations of geology, geomorphology, tectonics and gravity fields with a special focus on the geologically remarkable region of Pakistan: Sulaiman Fold Belt and Muslim Bagh ophiolite complex. This study presents new 12 thematic maps, which are technically made using scripting approaches and open tools. All maps cover the region of Pakistan and they are made using open source tools: GMT, R and QGIS. A GMT and R based scripting mapping is applied for mapping Pakistan, and its algorithm steps are presented stepwise as code snippets. A system complex approach of the data integration and formats reshaping, data conversion and reformatting for a single project of the geology of Pakistan is designed and developed based on the combination of the programming and scripting techniques and with additional QGIS based mapping, which effectively integrates the thematic geospatial multi-origin datasets. Various color palettes and cartographic visualization approaches have been used to achieve the best visualization. The resulting maps are explained and discussed. Correlation between spatial phenomena of Earth's gravity, geologic evolution and tectonic movements were pointed out and commented on. New 12 maps present the regional geologic setting of the country.

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    ZENODO
    Article . 2021
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    ZENODO
    Article . 2021
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    ePLUS
    Article . 2021
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    Authors: A. Ivčević; A. Ivčević; H. Mazurek; L. Siame; +7 Authors

    Code and data availability: The data set and software code are available at: https://doi.org/10.17605/OSF.IO/GMKYQ (Ivčević, 2021). Supplement: The supplement related to this article is available online at: https://doi.org/10.5194/nhess-21-3749-2021-supplement. Copyright © 2021 The Author(s). In order to mitigate the potentially dramatic effects of natural hazards, risk management measures are critical. However, the lack of interdisciplinary indicators and adaptable governance frameworks highlights society's vulnerability in the particular context of global environmental and climate change. This interdisciplinary research aimed at identifying reliable risk indicators and societal responses regarding natural hazards and climate change impacts to provide a governance framework for disaster risk reduction. Different societies face diverse risks and do not necessarily have the same level of local awareness of these risk. To explore the diversity of risks, two sites were selected from the Mediterranean basin, one chosen from the south coast (north Morocco) and the other from the north coast (the Italian island of Sardinia). North Morocco, a region of multi-risks, is characterised by high demographic and economic pressures; west Sardinia has remarkable biodiversity of wetlands and is characterised by high environmental and agricultural pressures, which in both cases intensify the vulnerability of the coastal areas. Testing for the local population's preparedness for future financial protection allowed for discussing the importance of risk awareness sessions or activities as an indicator of risk management. The significance of risk awareness sessions is shown in a quantitative part of the study, and its importance is also discussed with local stakeholders in north Morocco in a qualitative part of the study. It is shown that, although risk awareness sessions are recognised as important in risk management, they are not necessarily implemented. Based on these findings, further ideas on a new series of less descriptive, more dynamic and more user-friendly indicators are suggested. How can risk sessions be a dynamic indicator of a resilient society? The obtained results could serve in future governance frameworks for the mitigation of natural hazards in the Mediterranean region and more widely. Finally, the urgent need for continuous work to overcome the communication gap between the scientific community, risk administrators, civil society and the general population is emphasised. H2020 Marie Skłodowska-Curie Actions (grant no. 713750), the Regional Council of Provence–Alpes–Côte d’Azur and the Agence Nationale de la Recherche (grant nos. ANR-11-IDEX-0001-02, ANR-11-LABE-0061 and ANR-1-1E-0001-02).

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    Authors: Rivera-Torrente, M; Kroon, D; Coulet, M V; Marquez, C; +8 Authors

    AbstractUnderstanding the impact of shaping processes on solid adsorbents is critical for the implementation of MOFs in industrial separation processes or as catalytic materials. Production of MOF‐containing shaped particles is typically associated with loss of porosity and modification of acid sites, two phenomena that affect their performance. Herein, we report a detailed study on how extrusion affects the crystallinity, porosity, and acidity of the aluminium fumarate MOF with clays or SiO2 gel binders. Thorough characterization showed that the clay binders confer the extrudates a good mechanical robustness at the expense of porosity, while silica gel shows an opposite trend. The CO2 selectivity towards CH4, of interest for natural gas separation processes, is maintained upon the extrusion process. Moreover, probe FTIR spectroscopy revealed no major changes in the types of acid sites. This study highlights that these abundant and inexpensive clay materials may be used for scaling MOFs as active adsorbents.

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    Lirias
    Article . 2021
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    Chemistry - A European Journal
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    Chemistry - A European Journal
    Article . 2022
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    Chemistry - A European Journal
    Article . 2021 . Peer-reviewed
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ NARCISarrow_drop_down
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      Lirias
      Article . 2021
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      Chemistry - A European Journal
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      Chemistry - A European Journal
      Article . 2022
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      Chemistry - A European Journal
      Article . 2021 . Peer-reviewed
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    Authors: Collaboration, Super-Kamiokande; Abe, K.; Bronner, C.; Hayato, Y.; +196 Authors

    A new search for the diffuse supernova neutrino background (DSNB) flux has been conducted at Super-Kamiokande (SK), with a $22.5\times2970$-kton$\cdot$day exposure from its fourth operational phase IV. The new analysis improves on the existing background reduction techniques and systematic uncertainties and takes advantage of an improved neutron tagging algorithm to lower the energy threshold compared to the previous phases of SK. This allows for setting the world's most stringent upper limit on the extraterrestrial $\bar{\nu}_e$ flux, for neutrino energies below 31.3 MeV. The SK-IV results are combined with the ones from the first three phases of SK to perform a joint analysis using $22.5\times5823$ kton$\cdot$days of data. This analysis has the world's best sensitivity to the DSNB $\bar{\nu}_e$ flux, comparable to the predictions from various models. For neutrino energies larger than 17.3 MeV, the new combined $90\%$ C.L. upper limits on the DSNB $\bar{\nu}_e$ flux lie around $2.7$ cm$^{-2}$$\cdot$$\text{sec}^{-1}$, strongly disfavoring the most optimistic predictions. Finally, potentialities of the gadolinium phase of SK and the future Hyper-Kamiokande experiment are discussed. Comment: 42 pages, 37 figures, 14 tables

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    Biblos-e Archivo
    Other literature type . Article . 2021 . 2022 . Peer-reviewed
    License: APS Licenses for Journal Article Re-use
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    https://doi.org/10.48550/arxiv...
    Article . 2021
    License: CC BY
    Data sources: Datacite
    JAIRO
    Article . 2021
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    Hal-Diderot
    Article . 2021
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  • image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Authors: Gabriel Pasquet; Rokiya Houssein Hassan; Olivier Sissmann; Jacques Varet; +1 Authors

    Dihydrogen (H2) is generated by fluid–rock interactions along mid-ocean ridges (MORs) and was not, until recently, considered as a resource. However, in the context of worldwide efforts to decarbonize the energy mix, clean hydrogen is now highly sought after, and the production of natural H2 is considered to be a powerful alternative to electrolysis. The Afar Rift System has many geological features in common with MORs and offers potential in terms of natural H2 resources. Here, we present data acquired during initial exploration in this region. H2 contents in soil and within fumaroles were measured along a 200 km section across the Asal–Ghoubbet rift and the various intervening grabens, extending from Obock to Lake Abhe. These newly acquired data have been synthesized with existing data, including those from the geothermal prospect area of the Asal–Ghoubbet rift zone. Our results demonstrate that basalt alteration with oxidation of iron-rich facies and simultaneous reduction in water is the likely the source of the hydrogen, although H2S reduction cannot be ruled out. However, H2 volumes at the surface within fumaroles were found to be low, reaching only a few percent. These values are considerably lower than those found in MORs. This discrepancy may be attributed to bias introduced by surface sampling; for example, microorganisms may be preferentially consuming H2 near the surface in this environment. However, the low H2 generation rates found in the study area could also be due to a lack of reactants, such as fayalite (i.e., owing to the presence of low-olivine basalts with predominantly magnesian olivines), or to the limited volume and slow circulation of water. In future, access to additional subsurface data acquired through the ongoing geothermal drilling campaign will bring new insight to help answer these questions.

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    Geosciences
    Other literature type . Article . 2021 . Peer-reviewed
    License: CC BY
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    Geosciences
    Article
    License: CC BY
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    image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
    Geosciences
    Article . 2022
    Data sources: DOAJ-Articles
    DOAJ
    Article . 2021
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      image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Geosciencesarrow_drop_down
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      Geosciences
      Other literature type . Article . 2021 . Peer-reviewed
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      Geosciences
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      Geosciences
      Article . 2022
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    Authors: Aguilar, M.; Ali Cavasonza, Leila; Behlmann, M.; Laudi, E.; +197 Authors

    Physical review letters 127(27), 271102 (2021). doi:10.1103/PhysRevLett.127.271102 Published by APS, College Park, Md.

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    CERN Document Server
    Other literature type . 2021
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    Physical Review Letters
    Article . 2021
    Data sources: VIRTA
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    Physical Review Letters
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    Archive ouverte UNIGE
    Article . 2021
    License: CC BY
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    Physical Review Letters
    Article . 2021 . Peer-reviewed
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    image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
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    Article . 2021
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    UnissResearch
    Article . 2021
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      CERN Document Server
      Other literature type . 2021
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      Physical Review Letters
      Article . 2021
      Data sources: VIRTA
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      Physical Review Letters
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      Archive ouverte UNIGE
      Article . 2021
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      Physical Review Letters
      Article . 2021 . Peer-reviewed
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      Hal-Diderot
      Article . 2021
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      UnissResearch
      Article . 2021
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    Authors: Laura Martel; Thibault Charpentier; Pedro Amador Cedran; Chris Selfslag; +4 Authors

    In this study we reported the synthesis of three polycrystalline uranium borides UB1.78±0.02, UB3.61±0.041, and UB11.19±0.13 and their analyses using chemical analysis, X-ray diffraction, SQUID magnetometry, solid-state NMR, and Fourier transformed infrared spectroscopy. We discuss the effects of stoichiometry deviations on the lattice parameters and magnetic properties. We also provide their static and MAS-NMR spectra showing the effects of the 5f-electrons on the 11B shifts. Finally, the FTIR measurements showed the presence of a local disorder.

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    Minerals
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    DOAJ-Articles
    Article . 2022
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    Minerals
    Article . 2021 . Peer-reviewed
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      Minerals
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    Authors: D.-D. Rousseau; D.-D. Rousseau;

    When addressing the nature and origin of loess deposits and the associated environment as deduced from terrestrial mollusc faunas, Vojen Ložek produced a synthetic review of the state of the art at that time (Ložek, 1965a). This synthesis was one among several papers that he published the same year in English about “The loess environment in Central Europe” (Ložek, 1965c) or “Problems of analysis of the Quaternary nonmarine molluscan fauna in Europe” (Ložek, 1965b). It was mainly based on his own experience of investigating terrestrial molluscs in Czechoslovakian Quaternary deposits.

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    Copernicus Publications
    Other literature type . 2021
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    Eiszeitalter und Gegenwart
    Article
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    Eiszeitalter und Gegenwart
    Article . 2021 . Peer-reviewed
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    https://doi.org/10.7916/d8-6cw...
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    Authors: N. Deabji; N. Deabji; K. W. Fomba; S. El Hajjaji; +4 Authors

    Field measurements were conducted to determine aerosol chemical composition at a newly established remote high-altitude site in North Africa at the Atlas Mohammed V (AMV) atmospheric observatory located in the Middle Atlas Mountains. The main objectives of the present work are to investigate the variations in the aerosol composition and better assess global and regional changes in atmospheric composition in North Africa. A total of 200 particulate matter (PM10) filter samples were collected at the site using a high-volume (HV) collector in a 12 h sampling interval from August to December 2017. The chemical composition of the samples was analyzed for trace metals, water-soluble ions, organic carbon (OC/EC), aliphatic hydrocarbons, and polycyclic aromatic hydrocarbon (PAH) contents. The results indicate that high-altitude aerosol composition is influenced by both regional and transregional transport of emissions. However, local sources play an important role, especially during low wind speed periods, as observed for November and December. During background conditions characterized by low wind speeds (avg. 3 m s−1) and mass concentrations in the range from 9.8 to 12 µg m−3, the chemical composition is found to be dominated by inorganic elements, mainly suspended dust (61 %) and ionic species (7 %), followed by organic matter (7 %), water content (12 %), and unidentified mass (11 %). Despite the proximity of the site to the Sahara, its influence on the atmospheric composition at this high-altitude site was mainly seasonal and accounted for only 22 % of the sampling duration. Biogenic organics contributed up to 7 % of the organic matter with high contributions from compounds such as heneicosane, hentriacontane, and nonacosane. The AMV site is dominated by four main air mass inflows, which often leads to different aerosol chemical compositions. Mineral dust influence was seasonal and ranged between 21 % and 74 % of the PM mass, with peaks observed during the summer, and was accompanied by high concentrations of SO42- of up to 3.0 µg m−3. During winter, PM10 concentrations are low (<30 µg m−3), the influence of the desert is weaker, and the marine air masses (64 %) are more dominant with a mixture of sea salt and polluted aerosol from the coastal regions (Rabat and Casablanca). During the daytime, mineral dust contribution to PM increased by about 42 % because of road dust resuspension. In contrast, during nighttime, an increase in the concentrations of alkanes, PAHs, alkane-2-ones, and anthropogenic metals such as Pb, Ni, and Cu was found due to variations in the boundary layer height. The results provide the first detailed seasonal and diurnal variation of the aerosol chemical composition, which is valuable for long-term assessment of climate and regional influence of air pollution in North Africa.

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    Atmospheric Chemistry and Physics (ACP)
    Article . 2021 . Peer-reviewed
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      Atmospheric Chemistry and Physics (ACP)
      Article . 2021 . Peer-reviewed
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    Authors: Benjamin Pohl; Vincent Favier; Jonathan Wille; Danielle G. Udy; +8 Authors

    AbstractHere, we define weather regimes in the East Antarctica—Southern Ocean sector based on daily anomalies of 700 hPa geopotential height derived from ERA5 reanalysis during 1979–2018. Most regimes and their preferred transitions depict synoptic‐scale disturbances propagating eastwards off the Antarctic coastline. While regime sequences are generally short, their interannual variability is strongly driven by the polarity of the Southern Annular Mode (SAM). Regime occurrences are then intersected with atmospheric rivers (ARs) detected over the same region and period. ARs are equiprobable throughout the year, but clearly concentrate during regimes associated with a strong atmospheric ridges/blockings on the eastern part of the domain, which act to channel meridional advection of heat and moisture from the lower latitudes towards Antarctica. Both regimes and ARs significantly shape climate variability in Antarctica. Regimes favorable to AR occurrences are associated with anomalously warm and humid conditions in coastal Antarctica and, to a lesser extent, the hinterland parts of the Antarctic plateau. These anomalies are strongly enhanced during AR events, with warmer anomalies and dramatically amplified snowfall amounts. Large‐scale conditions favoring AR development are finally explored. They show weak dependency to the SAM, but particularly strong atmospheric ridges/blockings over the Southern Ocean appear as the most favorable pattern, in which ARs can be embedded, and to which they contribute.

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    Journal of Geophysical Research Atmospheres
    Article . 2021 . Peer-reviewed
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      Journal of Geophysical Research Atmospheres
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    Authors: Lemenkova, Polina;

    Zusammen mit der Entwicklung der Skripttechnologie in der Kartographie, wie den Generic Mapping Tools (GMT) und Bibliotheken der Programmiersprache R, wird die geologische und geophysikalische Kartierung energisch vorangetrieben, wobei die Integration der thematischen Daten, wie GEBCO/SRTM, EGM-2008 und offene geologische Raster- und Vektorschichten sind einer der primären Datensätze, die hochauflösende Rohquellen für die kartografische Visualisierung in geologisch komplexen Regionen wie Pakistan liefern. Diese Studie zielt darauf ab, Skriptmethoden der automatisierten Kartographie, Methoden der angewandten Geoinformatik für die geomorphometrische Analyse und technische Datenverarbeitung (Formatierung, Projektion, Darstellung) zu integrieren, um eine Synthese der geologischen, geophysikalischen und geomorphologischen Karten Pakistans als neue Informationen zur Unterstützung der Analyse bereitzustellen der georäumlichen Variationen von Geologie, Geomorphologie, Tektonik und Schwerkraftfeldern mit besonderem Schwerpunkt auf der geologisch bemerkenswerten Region Pakistan: Sulaiman Fold Belt und Muslim Bagh Ophiolith-Komplex. Diese Studie stellt neue 12 thematische Karten vor, die technisch mithilfe von Skriptansätzen und offenen Tools erstellt werden. Alle Karten decken die Region Pakistan ab und werden mit Open-Source-Tools erstellt: GMT, R und QGIS. Für die Kartierung Pakistans wird eine GMT- und R-basierte Skriptzuordnung angewendet, deren Algorithmusschritte schrittweise als Codeausschnitte dargestellt werden. Basierend auf der Kombination von Programmier- und Skripttechniken und mit zusätzlicher QGIS-basierter Kartierung wird ein systemkomplexer Ansatz zur Datenintegration und Formatumgestaltung, Datenkonvertierung und Neuformatierung für ein einzelnes Projekt zur Geologie Pakistans entworfen und entwickelt, das die Daten effektiv integriert thematische Geodatensätze mit mehreren Ursprüngen. Um die beste Visualisierung zu erreichen, wurden verschiedene Farbpaletten und kartografische Visualisierungsansätze verwendet. Die resultierenden Karten werden erklärt und diskutiert. Zusammenhänge zwischen räumlichen Phänomenen der Schwerkraft der Erde, geologischer Entwicklung und tektonischen Bewegungen wurden aufgezeigt und kommentiert. Neue 12 Karten präsentieren die regionale geologische Lage des Landes. Along with the development of the scripting technology in cartography, such as the Generic Mapping Tools (GMT) and libraries of R programming language, geologic and geophysical mapping is being vigorously promoted, where the integration of the thematic data, such as GEBCO/SRTM, EGM-2008 and open geological raster and vector layers is one of the primary datasets that provides the high- resolution raw sources for cartographic visualization in the geologically complex regions like Pakistan. This study aims to integrate scripting methods of automated cartography, methods of applied geoinformatics for geomorphometric analysis and technical data processing (formatting, projecting, plotting), to provide a synthesis of the geological, geophysical and geomorphological maps of Pakistan they as new information supporting analysis of the geospatial variations of geology, geomorphology, tectonics and gravity fields with a special focus on the geologically remarkable region of Pakistan: Sulaiman Fold Belt and Muslim Bagh ophiolite complex. This study presents new 12 thematic maps, which are technically made using scripting approaches and open tools. All maps cover the region of Pakistan and they are made using open source tools: GMT, R and QGIS. A GMT and R based scripting mapping is applied for mapping Pakistan, and its algorithm steps are presented stepwise as code snippets. A system complex approach of the data integration and formats reshaping, data conversion and reformatting for a single project of the geology of Pakistan is designed and developed based on the combination of the programming and scripting techniques and with additional QGIS based mapping, which effectively integrates the thematic geospatial multi-origin datasets. Various color palettes and cartographic visualization approaches have been used to achieve the best visualization. The resulting maps are explained and discussed. Correlation between spatial phenomena of Earth's gravity, geologic evolution and tectonic movements were pointed out and commented on. New 12 maps present the regional geologic setting of the country.

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    ZENODO
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    ePLUS
    Article . 2021
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      ZENODO
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    Authors: A. Ivčević; A. Ivčević; H. Mazurek; L. Siame; +7 Authors

    Code and data availability: The data set and software code are available at: https://doi.org/10.17605/OSF.IO/GMKYQ (Ivčević, 2021). Supplement: The supplement related to this article is available online at: https://doi.org/10.5194/nhess-21-3749-2021-supplement. Copyright © 2021 The Author(s). In order to mitigate the potentially dramatic effects of natural hazards, risk management measures are critical. However, the lack of interdisciplinary indicators and adaptable governance frameworks highlights society's vulnerability in the particular context of global environmental and climate change. This interdisciplinary research aimed at identifying reliable risk indicators and societal responses regarding natural hazards and climate change impacts to provide a governance framework for disaster risk reduction. Different societies face diverse risks and do not necessarily have the same level of local awareness of these risk. To explore the diversity of risks, two sites were selected from the Mediterranean basin, one chosen from the south coast (north Morocco) and the other from the north coast (the Italian island of Sardinia). North Morocco, a region of multi-risks, is characterised by high demographic and economic pressures; west Sardinia has remarkable biodiversity of wetlands and is characterised by high environmental and agricultural pressures, which in both cases intensify the vulnerability of the coastal areas. Testing for the local population's preparedness for future financial protection allowed for discussing the importance of risk awareness sessions or activities as an indicator of risk management. The significance of risk awareness sessions is shown in a quantitative part of the study, and its importance is also discussed with local stakeholders in north Morocco in a qualitative part of the study. It is shown that, although risk awareness sessions are recognised as important in risk management, they are not necessarily implemented. Based on these findings, further ideas on a new series of less descriptive, more dynamic and more user-friendly indicators are suggested. How can risk sessions be a dynamic indicator of a resilient society? The obtained results could serve in future governance frameworks for the mitigation of natural hazards in the Mediterranean region and more widely. Finally, the urgent need for continuous work to overcome the communication gap between the scientific community, risk administrators, civil society and the general population is emphasised. H2020 Marie Skłodowska-Curie Actions (grant no. 713750), the Regional Council of Provence–Alpes–Côte d’Azur and the Agence Nationale de la Recherche (grant nos. ANR-11-IDEX-0001-02, ANR-11-LABE-0061 and ANR-1-1E-0001-02).

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    Authors: Rivera-Torrente, M; Kroon, D; Coulet, M V; Marquez, C; +8 Authors

    AbstractUnderstanding the impact of shaping processes on solid adsorbents is critical for the implementation of MOFs in industrial separation processes or as catalytic materials. Production of MOF‐containing shaped particles is typically associated with loss of porosity and modification of acid sites, two phenomena that affect their performance. Herein, we report a detailed study on how extrusion affects the crystallinity, porosity, and acidity of the aluminium fumarate MOF with clays or SiO2 gel binders. Thorough characterization showed that the clay binders confer the extrudates a good mechanical robustness at the expense of porosity, while silica gel shows an opposite trend. The CO2 selectivity towards CH4, of interest for natural gas separation processes, is maintained upon the extrusion process. Moreover, probe FTIR spectroscopy revealed no major changes in the types of acid sites. This study highlights that these abundant and inexpensive clay materials may be used for scaling MOFs as active adsorbents.

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    Chemistry - A European Journal
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    Chemistry - A European Journal
    Article . 2022
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    Chemistry - A European Journal
    Article . 2021 . Peer-reviewed
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      Chemistry - A European Journal
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      Chemistry - A European Journal
      Article . 2022
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      Chemistry - A European Journal
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    Authors: Collaboration, Super-Kamiokande; Abe, K.; Bronner, C.; Hayato, Y.; +196 Authors

    A new search for the diffuse supernova neutrino background (DSNB) flux has been conducted at Super-Kamiokande (SK), with a $22.5\times2970$-kton$\cdot$day exposure from its fourth operational phase IV. The new analysis improves on the existing background reduction techniques and systematic uncertainties and takes advantage of an improved neutron tagging algorithm to lower the energy threshold compared to the previous phases of SK. This allows for setting the world's most stringent upper limit on the extraterrestrial $\bar{\nu}_e$ flux, for neutrino energies below 31.3 MeV. The SK-IV results are combined with the ones from the first three phases of SK to perform a joint analysis using $22.5\times5823$ kton$\cdot$days of data. This analysis has the world's best sensitivity to the DSNB $\bar{\nu}_e$ flux, comparable to the predictions from various models. For neutrino energies larger than 17.3 MeV, the new combined $90\%$ C.L. upper limits on the DSNB $\bar{\nu}_e$ flux lie around $2.7$ cm$^{-2}$$\cdot$$\text{sec}^{-1}$, strongly disfavoring the most optimistic predictions. Finally, potentialities of the gadolinium phase of SK and the future Hyper-Kamiokande experiment are discussed. Comment: 42 pages, 37 figures, 14 tables

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    https://doi.org/10.48550/arxiv...
    Article . 2021
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